Casting de Limitless
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Jake McDormanBrian Finch (22 ep.)
Jennifer CarpenterRebecca Harris (22 ep.)
Desmond HarringtonCasey Rooks (22 ep.)
Mary Elizabeth MastrantonioNasreen "Naz" Pouran (22 ep.)
Bradley CooperEdward Morra (22 ep.)
Hill HarperSpellman Boyle (22 ep.)
Ron RifkinDennis Finch (22 ep.)
Blair BrownMarie Finch (22 ep.)
Tom DegnanIke (22 ep.)
Michael James ShawMike (22 ep.)
Colin SalmonJarrod Sands (22 ep.)
Georgina HaigPiper Baird (22 ep.)
Megan GuinanRachel Finch (22 ep.)
Michael DevineJames "Tech" Padgett (22 ep.)
Charlie SemineFBI Agent (22 ep.)
Patch DarraghCameron Fish (5 ep.)
Frank AnelloFBI Agent (uncredited) (2 ep.)
Katelyn PearceOlivia (1 ep.)
Tyler RileyYoung Agent Ike (uncredited) (1 ep.)- Andrei AlorvskiAleksey Basayev (1 ep.)
- Anthony P. ThomasTrader Buddy (1 ep.)
Michelle Veintimillaava (1 ep.)
Evgeniya RadilovaIrina (1 ep.)
Victor CostaOfficer Rodriguez (1 ep.)
Adam KeaneYoung Brian (14 years old) (1 ep.)
Teresa Avia LimJogger (1 ep.)
Josh MoweryCongressman (uncredited) (1 ep.)- Raymond RichardsonHenry Watkins (uncredited) (1 ep.)
- Amanda TenenKayleigh (uncredited) (1 ep.)
Cooper AndrewsKenny Sumida (1 ep.)