Casting de The Testament of Sister New Devil
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Yūichi NakamuraBasara Tōjō (voice) (22 ep.)
朝井彩加Mio Naruse (voice) (22 ep.)
福原香織Maria Naruse (voice) (22 ep.)
Sarah Emi BridcuttYuki Nonaka (voice) (21 ep.)
Tomokazu SugitaYahiro Takigawa (voice) (17 ep.)
Keiji FujiwaraJin Tōjō (voice) (16 ep.)
吉田聖子Zest (voice) (16 ep.)
浅川悠Chisato Hasegawa (voice) (14 ep.)
野水伊織Kurumi Nonaka (voice) (14 ep.)- Tomokazu SugitaLars (voice) (8 ep.)
Kenjirō TsudaMamoru Sakazaki (voice) (6 ep.)
佳月大人Zolgia (voice) (5 ep.)
藏合紗恵子Shiho Aikawa (voice) (5 ep.)
味里Chika Sakaki (voice) (5 ep.)
Kazuyuki OkitsuLeoheart (voice) (5 ep.)
西原久美子Sheera (voice) (5 ep.)- Tomokazu SugitaWhite Mask (voice) (4 ep.)
Tesshô GendaRamusas (voice) (4 ep.)
楠大典Gald (voice) (4 ep.)
平川大輔Shiba Kyōichi (voice) (3 ep.)
井上剛Takashi Hayase (voice) (3 ep.)
富樫美鈴Childhood Basara (voice) (3 ep.)- Hiroki EtouShōhei Donoue (voice) (3 ep.)
田野アサミNanao Tachibana (voice) (3 ep.)
村瀬歩Luca (voice) (3 ep.)
山村響Lucia (voice) (3 ep.)
板取政明Kraus (voice) (3 ep.)
美名Noel (voice) (3 ep.)
乃村健次Volga (voice) (2 ep.)
喜多丘千陽Childhood Takashi (voice) (2 ep.)
嶋村侑Rikka Kajiura (voice) (2 ep.)
中川慶一Balflear (voice) (2 ep.)- Kenjirō TsudaOrnis (voice) (2 ep.)
- Reina KimuraFemale Student (voice) (2 ep.)
荒井勇樹Soldier (voice) (2 ep.)
Chika AnzaiFio (voice) (2 ep.)- Hiroki EtouBad A (voice) (1 ep.)
- 板取政明Bad B (voice) (1 ep.)
矢野正明Bad C (voice) (1 ep.)
白川周作Bad D (voice) (1 ep.)- Reina KimuraFemale Voice (voice) (1 ep.)
大下菜摘Female Student (voice) (1 ep.)- 矢野正明Announcement (voice) (1 ep.)
- Hiroki EtouSeito (voice) (1 ep.)
- 板取政明Elder (voice) (1 ep.)
- 金子修Man (voice) (1 ep.)
- 矢野正明Man (voice) (1 ep.)
衣川里佳Woman (voice) (1 ep.)- 矢野正明Kaiji Hozumi (voice) (1 ep.)
- Reina KimuraWoman (voice) (1 ep.)
- 板取政明Byakko (voice) (1 ep.)
有賀由樹子Female Teacher (voice) (1 ep.)- Hiroki EtouStudent (voice) (1 ep.)
- 矢野正明Student (voice) (1 ep.)
- Reina KimuraStudent (voice) (1 ep.)
- 美名Mio's Mother (voice) (1 ep.)
- 板取政明Mio's Father (voice) (1 ep.)
- Hiroki EtouMonster (voice) (1 ep.)
Kazuhiro SunsekiMale Student (voice) (1 ep.)- 矢野正明Train Announcement (voice) (1 ep.)
- Reina KimuraExecutive Committee (voice) (1 ep.)
亀山雄慈Commentator (voice) (1 ep.)
柏野昌俊Male Student (voice) (1 ep.)
角田雄二郎Male Student (voice) (1 ep.)
村上聡Male Student (voice) (1 ep.)
橘潤二Soldier (voice) (1 ep.)- Hiroki EtouSoldier (voice) (1 ep.)
- 矢野正明Soldier (voice) (1 ep.)
- Reina KimuraMaid (voice) (1 ep.)
荻野晴朗Nebula (voice) (1 ep.)
相楽信頼Soldier (voice) (1 ep.)
Kikuko InoueLiala (voice) (1 ep.)